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- W3160147212 abstract "Sn-based perovskite material has been selected as a strong contender for perovskite solar cells (PSCs) application compared with Pb-based perovskite, due to its more suitable bandgap and excellent optoelectronic characteristics. However, the poor quality of Sn-based perovskite film and the oxidation of Sn 2+ still lead to the unsatisfactory efficiency and instability of PSCs. In our work, a type of ligand “Trifluoroethylamine iodide (3FEAI)” was developed to achieve the crystallization regulation of FASnI 3 perovskite films, which could effectively improve the film quality while restricting the film defects. Moreover, it is found that the short-chain 3FEAI exhibited the better assistance of charge transport effect compared with the conventional ligand PEAI, which further contributed to the efficiency of PSCs. At last, with the introduction of 3FEAI, the prepared device shows the considerable efficiency (9.34%) and long-term stability (~10% PCE loss after 500 h of aging). • Considerable efficiency and light aging stability performance in Sn-based PSCs application. • Perovskite films with improved crystallinity and morphology were obtained by introducing 3FEAI ligands. • Less resistance for charge-exchanging on perovskite GBs/surface compared with the previous long-chain ligand." @default.
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- W3160147212 date "2021-09-01" @default.
- W3160147212 modified "2023-10-14" @default.
- W3160147212 title "High efficient and stable Tin-based perovskite solar cells via short-chain ligand modification" @default.
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- W3160147212 doi "https://doi.org/10.1016/j.orgel.2021.106198" @default.
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