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- W3160588349 abstract "Conjugated rod–rod block copolymers (BCPs) are important semiconducting materials because they combine the unique microphase-separation characteristics of BCPs with the remarkable optoelectronic properties of conjugated polymers. The ability to tailor the two fundamental phase transitions (microphase separation and crystallization) in BCPs could enable efficient control over their physical and optoelectronic properties. Herein, a set of poly(3-butylthiophene)-block-poly(3-dodecylthiophene) (P3BT-b-P3DDT) BCPs with controlled block ratios are synthesized and the interplay between their microphase separation and cocrystallization is explored by tuning both the intrinsic (i.e., block ratios) and extrinsic factors (i.e., solvent and thermal annealing temperatures). An increased P3BT content, slower solvent evaporation, and higher thermal annealing temperatures favor microphase separation in P3BT-b-P3DDT. Furthermore, the relationship between various P3BT-b-P3DDT crystalline structures and their charge-transport properties is scrutinized. This work elucidates how P3BT-b-P3DDT BCPs undergo microphase separation and crystallization and how these processes can be tailored, strengthening our fundamental understanding of conjugated rod–rod BCP systems." @default.
- W3160588349 created "2021-05-24" @default.
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- W3160588349 date "2021-05-10" @default.
- W3160588349 modified "2023-10-10" @default.
- W3160588349 title "Tailoring Cocrystallization and Microphase Separation in Rod–Rod Block Copolymers for Field-Effect Transistors" @default.
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- W3160588349 doi "https://doi.org/10.1021/acs.macromol.0c02788" @default.
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