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• W3160652004 abstract "When a low flux of time-frequency-entangled photon pairs (EPP) illuminates a two-photon transition, the rate of two-photon absorption (TPA) can be enhanced considerably by the quantum nature of photon number correlations and frequency correlations. We present a quantum-theoretic derivation of entangled TPA (ETPA) and calculate an upper bound on the amount of quantum enhancement that is possible in such systems. The derived bounds indicate that in order to observe ETPA the experiments would need to operate at a combination of significantly higher rates of EPP illumination, molecular concentrations, and conventional TPA cross sections than are achieved in typical experiments." @default.
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• W3160652004 date "2021-06-11" @default.
• W3160652004 modified "2023-10-02" @default.
• W3160652004 title "Quantifying the enhancement of two-photon absorption due to spectral-temporal entanglement" @default.
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• W3160652004 doi "https://doi.org/10.1364/oe.422544" @default.
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