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- W3161034395 abstract "The conventional (Zwanzig-Mountain) expressions for instantaneous elastic moduli of simple fluids predict their divergence as the limit of hard-sphere (HS) interaction is approached. However, elastic moduli of a true HS fluid are finite. Here we demonstrate that this paradox reveals the soft-to-hard-sphere crossover in fluid excitations and thermodynamics. With extensive in silico study of fluids with repulsive power-law interactions ($ensuremath{propto}{r}^{ensuremath{-}n}$), we locate the crossover at $nensuremath{simeq}10$--20 and develop a simple and accurate model for the HS regime. The results open prospects to deal with the elasticity and related phenomena in various systems, from simple fluids to melts and glasses." @default.
- W3161034395 created "2021-05-24" @default.
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- W3161034395 date "2021-05-13" @default.
- W3161034395 modified "2023-09-25" @default.
- W3161034395 title "From soft- to hard-sphere fluids: Crossover evidenced by high-frequency elastic moduli" @default.
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- W3161034395 doi "https://doi.org/10.1103/physreve.103.052117" @default.
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