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• W3161552480 endingPage "2100667" @default.
• W3161552480 startingPage "2100667" @default.
• W3161552480 abstract "Metal–CO2 batteries are among the most intriguing techniques for addressing the severe climate crisis and have matured significantly to simultaneously realize adequate fixation of CO2, energy storage, and conversion. Although significant efforts have been made, the practical application of metal–CO2 battery techniques is still restricted by various tremendous challenges, namely high charge potential, poor rate capability, and reversibility. This review seeks to present a realistic assessment of the most advanced metal–CO2 systems to identify problems, and opportunities to conquer these challenges. The recent progress on understanding the reaction mechanism of CO2 reduction/evolution, cathode materials, electrocatalysts design strategies, interface construction of metal anode/electrolyte, and the role of electrolytes are systematically reviewed and discussed. Meanwhile, high-performance electrode design principles and interface construction methods are also proposed. The effect of electrolyte and the difference between the nonaqueous and aqueous electrolyte systems in the context of the reaction mechanism, catalyst selection, metal anode protection, and corresponding enhancement strategies are also presented and evaluated. Finally, several perspectives on the opportunities and crucial challenges in the future development of metal–CO2 electrochemical systems for practical applications are proposed." @default.
• W3161552480 created "2021-05-24" @default.
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• W3161552480 creator A5085353152 @default.
• W3161552480 date "2021-05-13" @default.
• W3161552480 modified "2023-10-14" @default.
• W3161552480 title "Metal–CO ₂ Electrochemistry: From CO ₂ Recycling to Energy Storage" @default.
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