Matches in SemOpenAlex for { <https://semopenalex.org/work/W3162134296> ?p ?o ?g. }
- W3162134296 abstract "Abstract The understanding and rational design of heterogeneous catalysts for complex reactions, such as CO 2 reduction, requires knowledge of elementary steps and chemical species prevalent on the catalyst surface under operating conditions. Using in situ nanoscale surface-enhanced Raman scattering, we probe the surface of a Ag nanoparticle during plasmon-excitation-driven CO 2 reduction in water. Enabled by the high spatiotemporal resolution and surface sensitivity of our method, we detect a rich array of C 1 –C 4 species formed on the photocatalytically active surface. The abundance of multi-carbon compounds, such as butanol, suggests the favorability of kinetically challenging C–C coupling on the photoexcited Ag surface. Another advance of this work is the use of isotope labeling in nanoscale probing, which allows confirmation that detected species are the intermediates and products of the catalytic reaction rather than spurious contaminants. The surface chemical knowledge made accessible by our approach will inform the modeling and engineering of catalysts." @default.
- W3162134296 created "2021-05-24" @default.
- W3162134296 creator A5010803216 @default.
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- W3162134296 creator A5030902865 @default.
- W3162134296 creator A5037455068 @default.
- W3162134296 creator A5063852444 @default.
- W3162134296 date "2021-05-10" @default.
- W3162134296 modified "2023-10-17" @default.
- W3162134296 title "A rich catalog of C–C bonded species formed in CO2 reduction on a plasmonic photocatalyst" @default.
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