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- W3163057170 abstract "Abstract More than 3900 crystalline borates, including borate minerals and synthetic inorganic borates, in addition to a wealth of industrially-important boron-containing glasses, have been discovered and characterized. Of these compounds, 99.9 % contain only the traditional triangular BO 3 and tetrahedral BO 4 units, which polymerize into superstructural motifs. Herein, a mixed metal K 5 Ba 2 (B 10 O 17 ) 2 (BO 2 ) with linear BO 2 structural units was obtained, pushing the boundaries of structural diversity and providing a direct strategy toward the maximum thresholds of birefringence for optical materials design. 11 B solid-state nuclear magnetic resonance (NMR) is a ubiquitous tool in the study of glasses and optical materials; here, density functional theory-based NMR crystallography guided the direct characterization of BO 2 structural units. The full anisotropic shift and quadrupolar tensors of linear BO 2 were extracted from K 5 Ba 2 (B 10 O 17 ) 2 (BO 2 ) containing BO 2 , BO 3 , and BO 4 and serve as guides to the identification of this powerful moiety in future and, potentially, previously-characterized borate minerals, ceramics, and glasses." @default.
- W3163057170 created "2021-05-24" @default.
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- W3163057170 date "2021-05-10" @default.
- W3163057170 modified "2023-10-06" @default.
- W3163057170 title "Expanding the chemistry of borates with functional [BO2]− anions" @default.
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- W3163057170 doi "https://doi.org/10.1038/s41467-021-22835-4" @default.
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