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• W3163783556 abstract "Photocatalytic water splitting offers an economic and sustainable pathway for producing hydrogen as a zero-emission fuel, but it still suffers from low efficiencies limited by visible-light absorption capacity and charge separation kinetics. Herein, we report an interface-engineered 2D-C3N4/NiFe layered double hydroxide (CN/LDH) heterostructure that shows highly enhanced photocatalytic hydrogen evolution reaction (HER) rate with excellent long-term stability. The morphology and band gap structure of NiFe-LDH are precisely regulated by employing NH4F as a structure-directing agent, which enables a fine interfacial tuning via coupling with 2D-C3N4. The formation of a type II interface in CN/LDH enlarges the active surface area and promotes the charge separation efficiency, leading to an HER rate of 3087 μmol g-1 h-1, which is 14 times higher than that of 2D-C3N4. This study highlights a rational interface engineering strategy for the formation of a heterostructure with a proper hole transport co-catalyst for designing effective water-splitting photocatalysts." @default.
• W3163783556 created "2021-05-24" @default.
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• W3163783556 date "2021-05-19" @default.
• W3163783556 modified "2023-10-16" @default.
• W3163783556 title "Interface Engineering of a 2D-C₃N₄/NiFe-LDH Heterostructure for Highly Efficient Photocatalytic Hydrogen Evolution" @default.
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• W3163783556 doi "https://doi.org/10.1021/acsami.1c03240" @default.
• W3163783556 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34009942" @default.
• W3163783556 hasPublicationYear "2021" @default.
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