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• W3163998071 endingPage "16998" @default.
• W3163998071 startingPage "16994" @default.
• W3163998071 abstract "Abstract Atomically precise silver (Ag) nanoclusters are promising materials as catalysts, photocatalysts, and sensors because of their unique structures and mixed‐valence states (Ag + /Ag 0 ). However, their low stability hinders the in‐depth study of their intrinsic reactivity and catalytic property accompanying their redox processes. Herein, we demonstrate that a molecular hybrid of an atomically precise {Ag 27 } 17+ nanocluster and polyoxometalates (POMs) can efficiently cleave H 2 into protons and electrons. The Ag nanocluster accommodates electrons through the redox reaction from {Ag 27 } 17+ to {Ag 27 } 13+ , and the POM ligands play the following important roles: (i) a significant stabilization of the typically unstable Ag nanocluster to preserve its structure during the redox reaction with H 2 , (ii) formation of a unique interface between the Ag nanocluster and metal oxides for efficient H 2 cleavage, and (iii) storage of the generated protons on the negatively charged basic surface." @default.
• W3163998071 created "2021-06-07" @default.
• W3163998071 creator A5006226044 @default.
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• W3163998071 creator A5043858066 @default.
• W3163998071 creator A5050364079 @default.
• W3163998071 creator A5057650520 @default.
• W3163998071 date "2021-06-26" @default.
• W3163998071 modified "2023-10-15" @default.
• W3163998071 title "A Molecular Hybrid of an Atomically Precise Silver Nanocluster and Polyoxometalates for H₂ Cleavage into Protons and Electrons" @default.
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• W3163998071 doi "https://doi.org/10.1002/anie.202106786" @default.
• W3163998071 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34051034" @default.
• W3163998071 hasPublicationYear "2021" @default.
• W3163998071 type Work @default.
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