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• W3164181814 abstract "As one of the CO2 capture and utilization technologies, Li-CO2 batteries have attracted special interest in the application of carbon neutral. However, the design and fabrication of a low-cost high-efficiency cathode catalyst for reversible Li2CO3 formation and decomposition remains challenging. Here, guided by theoretical calculations, CO2 was utilized to activate the catalytic activity of conventional nitrogen-doped graphene, in which pyridinic-N and pyrrolic-N have a high total content (72.65%) and have a high catalytic activity in both CO2 reduction and evolution reactions, thus activating the reversible conversion of Li2CO3 formation and decomposition. As a result, the designed cathode has a low voltage gap of 2.13 V at 1200 mA g-1 and long-life cycling stability with a small increase in the voltage gap of 0.12 V after 170 cycles at 500 mA g-1. Our work suggests a way to design metal-free catalysts with high activity that can be used to activate the performance of Li-CO2 batteries." @default.
• W3164181814 created "2021-06-07" @default.
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• W3164181814 date "2021-05-25" @default.
• W3164181814 modified "2023-10-16" @default.
• W3164181814 title "Engineering the Active Sites of Graphene Catalyst: From CO₂ Activation to Activate Li-CO₂ Batteries" @default.
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• W3164181814 doi "https://doi.org/10.1021/acsnano.1c00756" @default.
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