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• W3165302533 endingPage "18808" @default.
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• W3165302533 abstract "The heterogeneous catalytic conversion of pollutants into useful industrial compounds is a two-goals at once process, which is highly recommended from the environmental, economic, and industrial points of view. In this regard, design materials with high conversion ability for a specific application is required to achieve such a goal. Herein, the synthesis conditions for the fabrication of BiPO4 nanorod bundles supported on g-C3N4 nanosheets as heterojunction composites was achieved using a facile ex situ chemical deposition for the reductive conversion of carcinogenic 4-nitrophenol (4-NP) into 4-aminophenol (4-AP). To better understand the mechanistic reduction pathways, BiPO4/g-C3N4 composites with varying ratios where obtained. The morphology and structure of BiPO4/g-C3N4 composites were checked using several methods: XRD, FE-SEM, HRTEM, XPS, and FT-IR, and it was found that hexagonal phase BiPO4 nanorod bundles were randomly distributed on the g-C3N4 nanosheets. Overall, the reduction ability of BiPO4/g-C3N4 composites was far better than bare BiPO4 and g-C3N4. A total reductive conversion of 4-NP at a concentration of 10 mg L-1 into 4-AP was found with 50% BiPO4/g-C3N4 composite within only one minute of reaction. Moreover, the presence of reducing agent (NaBH4) enhanced the kinetic rate constant up to 2.914 min-1 using 50% BiPO4/g-C3N4, which was much faster than bare BiPO4 (0.052 min-1) or g-C3N4 (0.004 min-1). The effects of some operating parameters including the initial concentration of 4-NP and catalyst dosage were also evaluated during the experiments. BiPO4/g-C3N4 showed great stability and recyclability, wherein, the catalytic reduction efficiency remains the same after five runs. A plausible 4-NP reduction mechanism was discussed. The high catalytic activity with the good stability of BiPO4/g-C3N4 make it a potential candidate for the reduction of nitroaromatic compounds in real wastewaters." @default.
• W3165302533 created "2021-06-07" @default.
• W3165302533 creator A5052140677 @default.
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• W3165302533 date "2021-01-01" @default.
• W3165302533 modified "2023-10-12" @default.
• W3165302533 title "Ultrafast conversion of carcinogenic 4-nitrophenol into 4-aminophenol in the dark catalyzed by surface interaction on BiPO₄/g-C₃N₄ nanostructures in the presence of NaBH₄" @default.
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• W3165302533 doi "https://doi.org/10.1039/d1ra02852a" @default.
• W3165302533 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35478611" @default.
• W3165302533 hasPublicationYear "2021" @default.
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