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• W3165348542 abstract "Abstract The oxidative dehydrogenation of ethane using CO 2 as soft oxidant for the production of ethylene, possesses the features of valorization of light alkane and utilization of greenhouse gas. Although a significant challenge, the control of the reaction extent can provide a potential on‐purpose ethylene technology. In the present paper, CeO 2 is proposed to be a promising catalyst, while the deep oxidation process of dry reforming is preferred. The SiO 2 coated CeO 2 catalyst can render the reaction more selective towards ethylene. Through high sensitivity low energy ion scattering spectroscopy, findings were made that SiO 2 only partially covered CeO 2 in the Si 0.1 CeO 2 sample, in which the ethylene selectivity was 2.7 times as high as that of the bulk CeO 2 based on the same conversion level. Further, density functional theory calculations also demonstrated that the presence of the SiO 2 layer was more conducive to the desorption of ethylene." @default.
• W3165348542 created "2021-06-07" @default.
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• W3165348542 date "2021-06-10" @default.
• W3165348542 modified "2023-10-14" @default.
• W3165348542 title "Porous Silica Coated Ceria as a Switch in Tandem Oxidative Dehydrogenation and Dry Reforming of Ethane with CO₂" @default.
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• W3165348542 doi "https://doi.org/10.1002/cctc.202100364" @default.
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