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- W3165585702 abstract "Chapter 1: A review of Shapiro reactions as a couplingstrategy in natural product total synthesis. The syntheses oflycoramine, galanthamine, yuehchukene analogues, ovalicin, studiestoward the ingenol core, haemanthidine, pretazettine, tazettine,crinamine, Taxol, colombiasin A, elisapterosin B, the AB ringfragment of spongistatin 1 and 8-epipuupewhedione are discussed.Chapter 2: The convergent total synthesis of the marine naturalproduct norrisolide is described. Both subunits, the hydrindanecore and the norrisane side chain, are prepared in an asymmetricfashion through kinetic resolution and enantioselectivecyclopropanation, respectively. A Shapiro reaction couples the twofragments and a Peterson olefination installs the 1,1-disubstitutedolefin. Chapter 3: Preliminary experiments to isolate thebiological target of norrisolide through reductive alkylation andtritium labeling are investigated. Further experiments are proposedto shed light on the primary norrisolide-proteininteractions." @default.
- W3165585702 created "2021-06-07" @default.
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- W3165585702 date "2009-01-01" @default.
- W3165585702 modified "2023-09-27" @default.
- W3165585702 title "Norrislide: Convergent Total Synthesis and PreliminaryBiological Investigations" @default.
- W3165585702 hasPublicationYear "2009" @default.
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