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- W3166123150 abstract "• Ultrathin graphitic carbon nitride (g-C3N4) nanosheets were prepared by the glucose assisted exfoliation of the bulk g-C3N4. • The product retained the basic structure and optical properties of g-C3N4 and is fully characterized. • The product showed excellent photocatalytic performance in the visible region, which was 4 times better than the bulk. • The introduction of ultrathin structure changed the H2O2 generation pathway from a two-step single-electron reduction to a one-step two-electron reduction. Photocatalytic generation of hydrogen peroxide (H 2 O 2 ) is a sustainable technique to realize the solar-energy conversion. Here, ultrathin graphitic carbon nitride (g-C 3 N 4 ) nanoplates with thickness of 1–3 nm was introduced for the efficient H 2 O 2 production. The as-obtained nanoplates demonstrated the H 2 O 2 production rate of 43.07 μmol g −1 h −1 and about 4 times as high as the pristine g-C 3 N 4 . Experimental results reflected that the ultrathin morphology offered an increased surface area, more active sites, smaller charge transfer length and stronger redox ability than that of the bulk counterparts. Moreover, the introduction of ultrathin structure switched the H 2 O 2 production pathway from a two-step single-electron reduction to a one-step two-electron reduction route. This study offered the deep elucidation of the influence of ultrathin structure on the photoactivity of semiconductor photocatalysts." @default.
- W3166123150 created "2021-06-22" @default.
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- W3166123150 date "2021-12-01" @default.
- W3166123150 modified "2023-10-12" @default.
- W3166123150 title "Fabrication of ultra-thin g-C3N4 nanoplates for efficient visible-light photocatalytic H2O2 production via two-electron oxygen reduction" @default.
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- W3166123150 doi "https://doi.org/10.1016/j.cej.2021.130615" @default.
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