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- W3166133023 abstract "The specific heat capacity $c_v$ of glass formers undergoes a hysteresis when subjected to a cooling-heating cycle, with a larger $c_v$ and a more pronounced hysteresis for fragile glasses than for strong ones. Here, we show that these experimental features, including the unusually large magnitude of $c_v$ of fragile glasses, are well reproduced by kinetic Monte Carlo and equilibrium study of a distinguishable particle lattice model (DPLM) incorporating a two-state picture of particle interactions. The large $c_v$ in fragile glasses is caused by a dramatic transfer of probabilistic weight from high-energy particle interactions to low-energy ones as temperature decreases." @default.
- W3166133023 created "2021-06-22" @default.
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- W3166133023 date "2021-08-25" @default.
- W3166133023 modified "2023-09-23" @default.
- W3166133023 title "Large heat-capacity jump in cooling-heating of fragile glass from kinetic Monte Carlo simulations based on a two-state picture" @default.
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- W3166133023 doi "https://doi.org/10.1103/physreve.104.024131" @default.
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