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- W3166621713 abstract "Terahertz Kerr effect technology, as a novel tool, is expected to study the low-frequency molecular dynamics of liquids since it can directly distinguish the time-resolved anisotropy information on the sub-picosecond scale. Here, this technology is used to measure a variety of aqueous salt solutions and observe the effects of different anions and cations on the structure and dynamics of water network. The obtained bipolar anisotropic response increases under the influence of multiple ions, which is mainly due to the energy transfer between the permanent dipole moment rotation of water molecules and the restricted translational motion of adjacent water molecules with THz electric field excitation. The classic viscosity-related coefficient B is used to analyze the amplitude and characteristics of the obtained anisotropic response, which implies the relationship between the intermolecular hydrogen bond dynamics and the macroscopic thermodynamic properties in the ionic aqueous solution. This work provides a new perspective for observing the low-frequency molecular motion in aqueous salt solutions." @default.
- W3166621713 created "2021-06-22" @default.
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- W3166621713 date "2021-10-01" @default.
- W3166621713 modified "2023-10-17" @default.
- W3166621713 title "Strong anisotropy in aqueous salt solutions revealed by terahertz-induced Kerr effect" @default.
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- W3166621713 doi "https://doi.org/10.1016/j.optcom.2021.127192" @default.
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