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• W3167351611 endingPage "106225" @default.
• W3167351611 startingPage "106225" @default.
• W3167351611 abstract "Extensive research efforts are devoted into seeking the thermally and mechanically durable dielectric materials for flexible electronics. In this work, a series of sulfonylated poly (phenylene ether)s (PPEs) were synthesized and served as gate dielectrics in the flexible OFET devices with crosslinked poly (2-allyl-6-methylphenol-co-2,6-dimethylphenol) (APPE) as substrate. The chemical structure, thermal, morphology, and dielectric properties were investigated, and the corresponding OFET devices were accordingly fabricated and characterized. We found that the discrepancy in sulfone content of PPE-xS renders the difference in thermal stability, surface polarity and dielectric constants. Among them, PPE-9kS with the highest sulfone content of 63% shows the best dielectric properties in the flexible OFET devices with hole mobility (μp) of 0.45 cm2 V−1 s−1, outperforming its parent polymer without sulfone group (PPE-9k) with μp of 0.14 cm2 V−1 s−1. Besides, the flexible device with PPE-9kS as dielectric exhibits highly retained device performance after cyclic bending or thermal treatment, which indicates the decent mechanical and thermal durability. The present study documents a practical methodology to fabricate a high-performance flexible OFET with excellent thermal and mechanical stability." @default.
• W3167351611 created "2021-06-22" @default.
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• W3167351611 date "2021-09-01" @default.
• W3167351611 modified "2023-10-12" @default.
• W3167351611 title "Functionalized Poly(phenylene ether) with high thermal stability as flexible dielectrics and substrates for organic field-effect transistors" @default.
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• W3167351611 doi "https://doi.org/10.1016/j.orgel.2021.106225" @default.
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