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- W3167876204 abstract "Developing effective catalysts for the degradation of organic pollutants in the water as well as water-splitting for hydrogen production by using solar energy is a promising and green route for utilization and protection of water resources. In this study, a mesoporous TiO2/CeO2 (m-TiO2/CeO2) nanocomposite aerogel was prepared and defect-engineered using a facile sol-gel method assisted solvent exchange and hydrogenated thermal treatment. The hydrogenated black m-TiO2/CeO2 nanocomposite aerogel exhibits the enhanced photocatalytic activity in the degradation of Rhodamine B (Rh B) and water splitting under visible-light irradiation. The degradation rate of Rh B reached ~96.4% in 60 min, and the hydrogen-evolution rate reached ~182 mmol h−1g−1, which are far higher than those of air-annealed m-TiO2 sample. The photocatalytic enhancement mechanisms can be attributed to multiple strategies, such as the large specific surface area, the enhanced conductivity, the generation of self-doped defects in Z-scheme m-TiO2/TiO2-x/CeO2-x heterojunction, which are beneficial for providing more active sites, extending the absorption range of solar light, and suppressing the recombination of photo-excited carriers." @default.
- W3167876204 created "2021-06-22" @default.
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- W3167876204 date "2021-10-01" @default.
- W3167876204 modified "2023-10-18" @default.
- W3167876204 title "Photocatalytic enhancement using defect-engineered black mesoporous TiO2/CeO2 nanocomposite aerogel" @default.
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- W3167876204 doi "https://doi.org/10.1016/j.compositesb.2021.109037" @default.
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