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• W3169008714 abstract "Sulfur chemistry based on solid–liquid dissolution-deposition route inevitably encounters shuttle of lithium polysulfides, its parasitic interaction with lithium (Li) anode and flood electrolyte environment. The sulfurized pyrolyzed poly(acrylonitrile) (S@pPAN) cathode favors solid-solid conversion mechanism in carbonate ester electrolytes but fails to pair high-capacity Li anode. Herein, we rationally design a cation-solvent fully coordinated ether electrolyte to simultaneously resolve the problems of both Li anode and S@pPAN cathode. Raman spectroscopy reveals a highly suppressed solvent activity and a cation-solvent fully coordinated structure (molar ratio 1:1). Consequently, Li electrodeposit evolves into round-edged morphology, LiF-rich interphase, and high reversibility. Moreover, S@pPAN cathode inherits a neat solid-phase redox reaction and fully eliminated the dissolution of lithium polysulfides. Finally, we harvest a long-life Li-S@pPAN pouch cell with slight Li metal excessive (0.4 time) and ultra-lean electrolyte design (1 μL mgS−1), delivering 394 Wh kg−1 energy density based on electrodes and electrolyte mass." @default.
• W3169008714 created "2021-06-22" @default.
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• W3169008714 date "2021-07-01" @default.
• W3169008714 modified "2023-10-16" @default.
• W3169008714 title "Designing Cation–Solvent Fully Coordinated Electrolyte for High‐Energy‐Density Lithium–Sulfur Full Cell Based On Solid–Solid Conversion" @default.
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• W3169008714 doi "https://doi.org/10.1002/anie.202106788" @default.
• W3169008714 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34101315" @default.
• W3169008714 hasPublicationYear "2021" @default.
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