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• W3169222591 abstract "There is a need to better understand the mechanisms that govern gas evolution (i.e., desorption) from supersaturated solutions at elevated pressures for improved design and troubleshooting of gas–liquid separators used in the oil and gas industry. The rate of gas evolution is generally represented in terms of the mass transfer coefficient, which can be affected by the presence of chemical additives. In the oil and gas industry, a wide variety of chemical additives are used, such as demulsifiers, antifoamers, and corrosion inhibitors. Two different classes of chemical additives were evaluated in this work, Xiameter PMX-200 (silicone-based) and Synperonic PE/L61 (alcohol-based). The rate of gas evolution (volumetric mass transfer coefficient) was determined at two different mixing speeds (25 and 500 rpm). The impact of the chemical additive concentration (Xiameter PMX-200) on the volumetric mass transfer coefficient was investigated using Exxsol D-110 (model oil) at different concentrations, while Synperonic PE/L61 (alcohol-based) was investigated only at a concentration of 80 ppm in Exxsol D-110. The effect of chemical additives in crude oils was also investigated using two crude oils (Crude A and B). For the measurements with crude oil, the concentration of Xiameter PMX-200 (silicone-based) was 10 ppm and that of Synperonic PE/L61 (alcohol-based) was 80 ppm. Results showed that the addition of chemical additives did not affect the number of moles of methane solubilized into the crude and model oils. However, the addition of chemical additives reduced the volumetric mass transfer coefficient during absorption and desorption into/from the crude and model oils. Based on these data, we hypothesize that chemical additives can form a resistive layer (near the bulk liquid–gas interface), thereby causing a reduction in the volumetric mass transfer coefficient." @default.
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• W3169222591 date "2021-06-07" @default.
• W3169222591 modified "2023-09-24" @default.
• W3169222591 title "Impact of Chemical Additives on Gas Evolution Behavior in Supersaturated Solutions at Elevated Pressures" @default.
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• W3169222591 doi "https://doi.org/10.1021/acs.energyfuels.1c00782" @default.
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