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- W3169301251 abstract "Organic solar cells are approaching power conversion efficiencies of other thin-film technologies. However, in order to become truly market competitive, the still substantial voltage losses need to be reduced. Here, the synthesis and characterization of four novel arylamine-based push-pull molecular donors was described, two of them exhibiting a methyl group at the para-position of the external phenyl ring of the arylamine block. Assessing the charge-transfer state properties and the effects of methylation on the open-circuit voltage of the device showed that devices based on methylated versions of the molecular donors exhibited reduced voltage losses due to decreased non-radiative recombination. Modelling suggested that methylation resulted in a tighter interaction between donor and acceptor molecules, turning into a larger oscillator strength to the charge-transfer states, thereby ensuing reduced non-radiative decay rates." @default.
- W3169301251 created "2021-06-22" @default.
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- W3169301251 date "2021-06-29" @default.
- W3169301251 modified "2023-10-13" @default.
- W3169301251 title "Reducing Non‐Radiative Voltage Losses by Methylation of Push–Pull Molecular Donors in Organic Solar Cells" @default.
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- W3169301251 doi "https://doi.org/10.1002/cssc.202100799" @default.
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