Matches in SemOpenAlex for { <https://semopenalex.org/work/W3170172158> ?p ?o ?g. }
- W3170172158 endingPage "8670" @default.
- W3170172158 startingPage "8663" @default.
- W3170172158 abstract "Luminol-dissolved O2 electrochemiluminescence (ECL)-sensing platforms have been widely developed for sensitive and reliable detection, while their actual ECL mechanisms are still in controversy due to the involved multiple reactive oxygen species (ROS). Different from the structural complexity of nanomaterials, well-defined single-atom catalysts (SACs) as coreaction accelerators will provide great prospects for investigating the ECL mechanism at the atomic level. Herein, two carbon-supported nickel SACs with the active centers of Ni-N4 (Ni-N4/C) and Ni-N2O2 (Ni-N2O2/C) were synthesized as efficient coreaction accelerators to enhance the ECL signals of a luminol-dissolved O2 system. By modulating the surrounding environment of the center metal atoms, their corresponding oxygen reduction behaviors can be well controlled to selectively produce intermediate ROS, giving a great chance to study the following ECL process. According to the experimental and calculated results, the superoxide radical (O2•-) acts as the main radical for the ECL reaction and the Ni-N4/C catalyst with the four-electron pathway to activate dissolved O2 is preferential to enhance ECL emission." @default.
- W3170172158 created "2021-06-22" @default.
- W3170172158 creator A5001996060 @default.
- W3170172158 creator A5009348185 @default.
- W3170172158 creator A5024515567 @default.
- W3170172158 creator A5024591419 @default.
- W3170172158 creator A5024613158 @default.
- W3170172158 creator A5031722471 @default.
- W3170172158 creator A5033062026 @default.
- W3170172158 creator A5033880878 @default.
- W3170172158 creator A5056691753 @default.
- W3170172158 creator A5058895264 @default.
- W3170172158 creator A5089580445 @default.
- W3170172158 date "2021-06-08" @default.
- W3170172158 modified "2023-10-16" @default.
- W3170172158 title "Modulating Oxygen Reduction Behaviors on Nickel Single-Atom Catalysts to Probe the Electrochemiluminescence Mechanism at the Atomic Level" @default.
- W3170172158 cites W1982248426 @default.
- W3170172158 cites W1991048202 @default.
- W3170172158 cites W2047435229 @default.
- W3170172158 cites W2050762075 @default.
- W3170172158 cites W2056913972 @default.
- W3170172158 cites W2092157292 @default.
- W3170172158 cites W2143981217 @default.
- W3170172158 cites W2148284063 @default.
- W3170172158 cites W2165867195 @default.
- W3170172158 cites W2295376186 @default.
- W3170172158 cites W2318267179 @default.
- W3170172158 cites W2582514558 @default.
- W3170172158 cites W2624508105 @default.
- W3170172158 cites W2740830198 @default.
- W3170172158 cites W2776687276 @default.
- W3170172158 cites W2779891327 @default.
- W3170172158 cites W2790507915 @default.
- W3170172158 cites W2805573727 @default.
- W3170172158 cites W2809564681 @default.
- W3170172158 cites W2854976895 @default.
- W3170172158 cites W2924670559 @default.
- W3170172158 cites W2925286496 @default.
- W3170172158 cites W2935028938 @default.
- W3170172158 cites W2949881242 @default.
- W3170172158 cites W2969643625 @default.
- W3170172158 cites W2971217758 @default.
- W3170172158 cites W2971471509 @default.
- W3170172158 cites W2979525526 @default.
- W3170172158 cites W2979978014 @default.
- W3170172158 cites W2998370555 @default.
- W3170172158 cites W2999727704 @default.
- W3170172158 cites W3014910550 @default.
- W3170172158 cites W3017997820 @default.
- W3170172158 cites W3020718800 @default.
- W3170172158 cites W3028499025 @default.
- W3170172158 cites W3035556923 @default.
- W3170172158 cites W3037491188 @default.
- W3170172158 cites W3047119310 @default.
- W3170172158 cites W3047275156 @default.
- W3170172158 cites W3054337399 @default.
- W3170172158 cites W3112875897 @default.
- W3170172158 cites W3113447631 @default.
- W3170172158 cites W4232565521 @default.
- W3170172158 cites W4247733929 @default.
- W3170172158 doi "https://doi.org/10.1021/acs.analchem.1c01835" @default.
- W3170172158 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34100585" @default.
- W3170172158 hasPublicationYear "2021" @default.
- W3170172158 type Work @default.
- W3170172158 sameAs 3170172158 @default.
- W3170172158 citedByCount "43" @default.
- W3170172158 countsByYear W31701721582021 @default.
- W3170172158 countsByYear W31701721582022 @default.
- W3170172158 countsByYear W31701721582023 @default.
- W3170172158 crossrefType "journal-article" @default.
- W3170172158 hasAuthorship W3170172158A5001996060 @default.
- W3170172158 hasAuthorship W3170172158A5009348185 @default.
- W3170172158 hasAuthorship W3170172158A5024515567 @default.
- W3170172158 hasAuthorship W3170172158A5024591419 @default.
- W3170172158 hasAuthorship W3170172158A5024613158 @default.
- W3170172158 hasAuthorship W3170172158A5031722471 @default.
- W3170172158 hasAuthorship W3170172158A5033062026 @default.
- W3170172158 hasAuthorship W3170172158A5033880878 @default.
- W3170172158 hasAuthorship W3170172158A5056691753 @default.
- W3170172158 hasAuthorship W3170172158A5058895264 @default.
- W3170172158 hasAuthorship W3170172158A5089580445 @default.
- W3170172158 hasConcept C111335779 @default.
- W3170172158 hasConcept C111472728 @default.
- W3170172158 hasConcept C138885662 @default.
- W3170172158 hasConcept C147789679 @default.
- W3170172158 hasConcept C149635348 @default.
- W3170172158 hasConcept C161790260 @default.
- W3170172158 hasConcept C17525397 @default.
- W3170172158 hasConcept C178790620 @default.
- W3170172158 hasConcept C185592680 @default.
- W3170172158 hasConcept C2524010 @default.
- W3170172158 hasConcept C2992754303 @default.
- W3170172158 hasConcept C2994571290 @default.
- W3170172158 hasConcept C33923547 @default.
- W3170172158 hasConcept C38965407 @default.
- W3170172158 hasConcept C41008148 @default.
- W3170172158 hasConcept C504270822 @default.
- W3170172158 hasConcept C52859227 @default.