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• W3170461569 endingPage "111253" @default.
• W3170461569 startingPage "111253" @default.
• W3170461569 abstract "• A non-Born-Oppenheimer time-dependent Schrödinger equation is numerically solved to study the dissociative-ionization of H 2 + molecule subjected to strong field six-cycle laser pulses ( I = 4 × 10 14 W / cm 2 , λ = 800 nm ) . • Analysis of the time evolution of the H 2 + nuclear wave packet is performed using Floquet formalism in the adiabatic representation to gain newly insightful images of the nonlinear processes such as vibrational trapping, above-threshold dissociation, tunneling, and bond-softening of the laser-driven nuclear wave packet on two lowest field-dressed adiabatic potential energy curves. • Starting from an initial state-selected vibrational level of H 2 , the images enable ones to fully comprehend the dissociative-ionization dynamics of H 2 + , notably in the vicinity of a conical intersection up to eventually entering the two exit channels with the main one producing fragments H + H + via the H 2 + ( 2 ∑ u + ) exit channel. • The direct treatment of the electronic-nuclear wave packet of H 2 enables one to image the one-electron nuclear localization of H 2 + on the right or left of field-distorted double-well Coulomb potential to reveal the influence of the field on the charge-resonance enhanced ionization coupled with the other nonlinear processes. A non-Born–Oppenheimer time-dependent Schrödinger equation is numerically solved to study the dissociative-ionization of H 2 + subjected to strong field six-cycle laser pulses ( I = 4 × 10 14 W / cm 2 , λ = 800 nm ) . Analysis of the evolution of H 2 + nuclear wave packet is performed using Floquet formalism in the adiabatic representation to gain newly insightful images of the nonlinear processes in the vicinity of a conical intersection of two lowest field-dressed adiabatic states. The coherent superposition of the states leads to the right or left localization of H 2 + on the field-distorted double-well Coulomb potential." @default.
• W3170461569 created "2021-06-22" @default.
• W3170461569 creator A5067493222 @default.
• W3170461569 date "2021-09-01" @default.
• W3170461569 modified "2023-09-29" @default.
• W3170461569 title "Ultrafast quantum imaging in the dissociation of <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML altimg=si110.svg><mml:mrow><mml:msubsup><mml:mrow><mml:mi mathvariant=normal>H</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow><mml:mrow><mml:mo>+</mml:mo></mml:mrow></mml:msubsup></mml:mrow></mml:math> via the induced conical intersection of two lowest adiabatic states by strong field laser pulses" @default.
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• W3170461569 doi "https://doi.org/10.1016/j.chemphys.2021.111253" @default.
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