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• W3170483765 startingPage "130785" @default.
• W3170483765 abstract "The intriguing intrinsic photoluminescence (PL) properties of gold nanorods (AuNRs) have been intensively studied over the last years, not only in the linear but also in the non-linear optics regime, boosting their applicability in various fields of nanobiotechnology. In the present work, we investigate the two-photon excited (TPE) intrinsic PL of different-aspect ratio (AR) synthesized AuNRs, coated with gelatin ([email protected]), by performing innovative fluorescence spectroscopy - fluorescence lifetime imaging microscopy (FLIM) combined studies on individual [email protected] In the first step, we employ Finite-difference time-domain (FDTD) simulations to confirm the optical response of AuNRs before and after coating with gelatin. While TPE FLIM assays performed under 800 nm excitation expose some interesting aspect regarding the AR-dependent TPE PL emission generated by individual [email protected], spectroscopic measurements reveal that the TPE PL has a lifetime of around 100 ps and overlaps the corresponding transverse plasmonic band. Finally, we evaluate the effect of laser excitation power and wavelength on the TPE PL, pointing towards the important correlation between these parameters and the TPE PL performance of [email protected], as possible contrast agents for label-free TPE fluorescence imaging applications." @default.
• W3170483765 created "2021-06-22" @default.
• W3170483765 creator A5047367672 @default.
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• W3170483765 date "2021-11-01" @default.
• W3170483765 modified "2023-09-26" @default.
• W3170483765 title "Two-photon excited photoluminescence lifetime imaging studies on individual gelatin-coated gold nanorods" @default.
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• W3170483765 doi "https://doi.org/10.1016/j.molstruc.2021.130785" @default.
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