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- W3170901445 abstract "Traditional nanofiltration membranes (NFMs) formed by interfacial polymerization (IP) present relatively low water permeance due to the limitation of polymer-based supports. This work reports high-performance carbon nanotubes-polyamide (CNTs-PA) NFMs with interlayer and functional layer covalently coupled. These membranes feature an interpenetrating network structure, which leads to an extremely high Congo red rejection of 99.47%. The water permeance of the optimal membrane (48.98 L m-2h−1 bar−1) is much higher than most membranes with similar Congo red rejection. Meanwhile, the obtained membranes show an excellent selectivity to NaCl/dye mixed solution (the selectivity of NaCl/CR is 150.32). Moreover, this work comprehensively demonstrates the aggregation kinetics of dye molecules under different pH environments, which strongly affects the dye rejection of the CNTs-PA membrane. The membrane exhibits a switchable CR release property that the CR rejection is severely disabled (2.12%) under a strong alkaline environment and immediately re-effective (99.38%) after neutralization. Building on these findings, our work expands the possibilities of NFMs in ultrafast molecular sieving and pH-responsive separation." @default.
- W3170901445 created "2021-06-22" @default.
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- W3170901445 date "2021-12-01" @default.
- W3170901445 modified "2023-10-04" @default.
- W3170901445 title "Highly permeable carbon nanotubes/polyamide layered membranes for molecular sieving" @default.
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- W3170901445 doi "https://doi.org/10.1016/j.cej.2021.130684" @default.
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