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- W3170902911 abstract "Atomic-scale chemical modification of surface-adsorbed ethyl groups on Si(001) was induced and studied by means of scanning tunneling microscopy. Tunneling at sample bias > +1.5V leads to tip-induced C-H cleavage of a $beta$-hydrogen of the covalently bound ethyl configuration. The reaction is characterized by the formation of an additional Si-H and a Si-C bond. The reaction probability shows a linear dependence on the tunneling current at 300 K; the reaction is largely suppressed at 50 K. The observed tip-induced surface reaction at room temperature is thus attributed to a one-electron excitation in combination with thermal activation." @default.
- W3170902911 created "2021-06-22" @default.
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- W3170902911 date "2021-07-01" @default.
- W3170902911 modified "2023-10-08" @default.
- W3170902911 title "Tip-induced β -hydrogen dissociation in an alkyl group bound on Si(001)" @default.
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- W3170902911 doi "https://doi.org/10.1088/1361-648x/ac0a1c" @default.
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