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• W3171006985 abstract "Zeolite Li-X is considered the best adsorbent for air separation (i.e., N2/O2 one). However, this zeolite adsorbent suffers from serious limitations of preparation and process operation. Here, we report that Ag+-exchanged chabazite (Ag-CHA-6.0) with a Si/Al ratio of 6.0 shows comparable N2/O2 separation performance, but higher CO2 resistance than Li-X under N2/O2 simulated conditions. The characterization results reveal that its excellent separation performance may be due to the preferential formation of partially charged silver clusters (Agnδ+) within the CHA framework upon activation under a dynamic vacuum of 10−3 Torr at 523 K. The intrazeolitic formation of these Agnδ+ clusters, whose ability to form π-complexation with N2 is higher than monovalent silver ions, was found to depend not only on the structure type of the zeolite support, but also its framework Si/Al ratio." @default.
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• W3171006985 date "2021-08-01" @default.
• W3171006985 modified "2023-10-14" @default.
• W3171006985 title "Silver-exchanged CHA zeolite as a CO2-resistant adsorbent for N2/O2 separation" @default.
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• W3171006985 doi "https://doi.org/10.1016/j.micromeso.2021.111239" @default.
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