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• W3172529191 abstract "Here, we use x-rays to create and probe quantum coherence in the photoionized amino acid glycine. The outgoing photoelectron leaves behind the cation in a coherent superposition of quantum mechanical eigenstates. Delayed x-ray pulses track the induced coherence through resonant x-ray absorption that induces Auger decay and by photoelectron emission from sequential double photoionization. Sinusoidal temporal modulation of the detected signal at early times (0 to 25 fs) is observed in both measurements. Advanced ab initio many-electron simulations allow us to explain the first 25 fs of the detected coherent quantum evolution in terms of the electronic coherence. In the kinematically complete x-ray absorption measurement, we monitor its dynamics for a period of 175 fs and observe an evolving modulation that may implicate the coupling of electronic to vibronic coherence at longer time scales. Our experiment provides a direct support for the existence of long-lived electronic coherence in photoionized biomolecules." @default.
• W3172529191 created "2021-06-22" @default.
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• W3172529191 date "2022-06-03" @default.
• W3172529191 modified "2023-10-18" @default.
• W3172529191 title "Electronic quantum coherence in glycine molecules probed with ultrashort x-ray pulses in real time" @default.
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• W3172529191 doi "https://doi.org/10.1126/sciadv.abn6848" @default.
• W3172529191 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35648864" @default.
• W3172529191 hasPublicationYear "2022" @default.
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