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- W3172670837 abstract "Abstract A highly efficient, low-cost and environmentally friendly photocathode with long-term stability is the goal of practical solar hydrogen evolution applications. Here, we found that the Cu 3 BiS 3 film-based photocathode meets the abovementioned requirements. The Cu 3 BiS 3 -based photocathode presents a remarkable onset potential over 0.9 V RHE with excellent photoelectrochemical current densities (~7 mA/cm 2 under 0 V RHE ) and appreciable 10-hour long-term stability in neutral water solutions. This high onset potential of the Cu 3 BiS 3 -based photocathode directly results in a good unbiased operating photocurrent of ~1.6 mA/cm 2 assisted by the BiVO 4 photoanode. A tandem device of Cu 3 BiS 3 -BiVO 4 with an unbiased solar-to-hydrogen conversion efficiency of 2.04% is presented. This tandem device also presents high stability over 20 hours. Ultimately, a 5 × 5 cm 2 large Cu 3 BiS 3 -BiVO 4 tandem device module is fabricated for standalone overall solar water splitting with a long-term stability of 60 hours." @default.
- W3172670837 created "2021-06-22" @default.
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- W3172670837 date "2021-06-18" @default.
- W3172670837 modified "2023-10-16" @default.
- W3172670837 title "Wittichenite semiconductor of Cu3BiS3 films for efficient hydrogen evolution from solar driven photoelectrochemical water splitting" @default.
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- W3172670837 doi "https://doi.org/10.1038/s41467-021-24060-5" @default.
- W3172670837 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/8213846" @default.
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