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• W3173100718 abstract "The metallic phase of 1T-MoS2 nanoflowers (NFs) and the semiconducting phase of 2H-MoS2 NFs were prepared by a facile solvothermal and combustion method. The antibacterial activities, reactive oxygen species (ROS) generation, and light-driven antibacterial mechanism of metallic 1T-MoS2 NFs and semiconducting 2H-MoS2 NFs were demonstrated with the bacterium Escherichia coli (E. coli) under light irradiation. Results of the bacterial growth curve and ROS generation analyses revealed higher light-driven antibacterial activity of metallic 1T-MoS2 NFs compared to semiconducting 2H-MoS2 NFs. Electron paramagnetic resonance (EPR) spectroscopy demonstrated that the ROS of the superoxide anion radical •O2– was generated due to the incubation of 1T-MoS2 NFs and E. coli with light irradiation. Furthermore, E. coli incubated with metallic 1T-MoS2 NFs exhibited significant damage to the bacterial cell walls, complete bacterial destruction, and abnormal elongation after light irradiation. The light-driven antibacterial mechanism of metallic 1T-MoS2 NFs was examined, and we found that, under light irradiation, photoinduced electrons were generated by metallic 1T-MoS2 NFs, and then the photoinduced electrons reacted with oxygen to generate superoxide anion radical which induced bacterial death. For semiconducting 2H-MoS2 NFs, photoinduced electrons and holes rapidly recombined resulting in a decrease in ROS generation which diminished the light-driven antibacterial activity." @default.
• W3173100718 created "2021-06-22" @default.
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• W3173100718 date "2021-06-02" @default.
• W3173100718 modified "2023-10-18" @default.
• W3173100718 title "Phase-Dependent MoS₂ Nanoflowers for Light-Driven Antibacterial Application" @default.
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• W3173100718 doi "https://doi.org/10.1021/acssuschemeng.1c01868" @default.
• W3173100718 hasPublicationYear "2021" @default.
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