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• W3173454967 abstract "Hydrogen can be generated by the photolysis of water with semiconductors as photocatalysts. The most important characteristics of water splitting are its durability and efficiency. Furthermore, TiO2 and 3C–SiC are durable photocatalysts. Because of their different band gaps and conductivity types, a tandem structure combined with these materials functions as an efficient and durable solar water splitting system. It was observed that the photocurrent from the tandem structure was higher at low pH, as noted by the pH dependence of the photocurrent at the TiO2 photoanode. The photocurrent from the tandem structure had a light intensity dependence similar to the photocurrent from the TiO2 photoanode. Therefore, the performance of the tandem structure appears to be limited by the photocurrents from the TiO2 photoanode. We obtained a maximum applied bias photon-to-current conversion efficiency of approximately 0.74% from the tandem structure with no additional bias applied. We also confirmed the presence of a stable photocurrent from the tandem structure for over ~100 days." @default.
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• W3173454967 date "2021-09-01" @default.
• W3173454967 modified "2023-10-13" @default.
• W3173454967 title "Durable and efficient photoelectrochemical water splitting using TiO2 and 3C–SiC single crystals in a tandem structure" @default.
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• W3173454967 doi "https://doi.org/10.1016/j.solmat.2021.111260" @default.
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