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- W3174412941 abstract "The development of wearable electronics has led to new requirements for flexible and high-energy batteries. However, the conventional polyvinylidene fluoride binder fails in the manufacture of high-loaded and thick battery electrodes owing to its insufficient adhesiveness and electronic insulation, let alone for flexible devices. Furthermore, organic processing is expensive and not eco-friendly. Herein, the authors report a novel aqueous conductive binder made of carbon nanotubes interwoven in cellulose nanosheets, successfully satisfying the fabrication of flexible yet high-strength electrodes for universal active materials of different sizes, morphologies, and negative-to-positive working potentials, with a high mass loading of up to ≈90 mg cm−2. The conductive binder has an ultrathin 2D-reticular nanosheet structure that forms continuous conductive skeletons in electrodes to segregate and warp active particles via a robust “face-to-point” bonding mode, allowing the fabricated electrodes to have remarkable flexibility and excellent mechanical integrity even under various external forces and excessive electrolyte erosion. Flexible LCO cathodes with a mass loading of >30 mg cm−2 as a case study exhibit high mechanical strength (>20 MPa) and can easily achieve an ultrahigh areal capacity of 12.1 mAh cm−2. This cellulose-based binder system is ideal for advanced high-performance functional devices, especially for flexible and high-energy batteries." @default.
- W3174412941 created "2021-07-05" @default.
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- W3174412941 date "2021-06-17" @default.
- W3174412941 modified "2023-10-14" @default.
- W3174412941 title "A Universal Aqueous Conductive Binder for Flexible Electrodes" @default.
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- W3174412941 doi "https://doi.org/10.1002/adfm.202102284" @default.
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