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• W3174415181 endingPage "120481" @default.
• W3174415181 startingPage "120481" @default.
• W3174415181 abstract "Ligand-stabilized Bi nanosheets are obtained from in-situ electrochemical reduction of a Bi-based metal-organic framework, which exhibit remarkable electrocatalytic performance for CO 2 reduction. A high Faradic efficiency of 98 % for formate are achieved with an improved durability over 40 h, attributing to the abundant under-coordinated Bi active sites stabilized by residual organic ligands. • An in-situ formed Bi-molecular surface maximizes the under-coordinated surface atoms as catalytic active sites. • The hybrid surface improves the stability of Bi catalyst by suppressing the reconstruction of active sites. • The ligand-stabilized Bi nanosheets deliver a high formate Faradaic efficiency of 98 % and improved stability over 40 h. Electrochemical reduction of carbon dioxide provides a feasible solution to the energy and climate crisis. Bi-based catalysts are promising candidates to electrochemically convert carbon dioxide (CO 2 ) into formic acid or formate. Herein, ligand-stabilized Bi nanosheets are obtained from in-situ electrochemical reduction of a Bi-based metal-organic framework, which exhibit remarkable electrocatalytic performance for CO 2 reduction. A high Faradic efficiency of 98 % for formate is achieved at a potential of -0.80 V vs . reversible hydrogen electrode (RHE) with an improved durability over 40 h. The remarkable electrocatalytic activity and stability could be attributed to the in-situ generated catalyst with abundant under-coordinated Bi active sites, which are effectively stabilized by residual ligands adsorbed on surface. This study demonstrates that ligand-stabilized under-coordinated surface sites would be facilely generated from in-situ transformation of metal-organic precursors for highly efficient CO 2 conversion." @default.
• W3174415181 created "2021-07-05" @default.
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• W3174415181 date "2021-11-01" @default.
• W3174415181 modified "2023-10-17" @default.
• W3174415181 title "In-situ formation of ligand-stabilized bismuth nanosheets for efficient CO2 conversion" @default.
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• W3174415181 doi "https://doi.org/10.1016/j.apcatb.2021.120481" @default.
• W3174415181 hasPublicationYear "2021" @default.
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