FRINK Linked Data Fragments server

Matches in SemOpenAlex for { <https://semopenalex.org/work/W3176202430> ?p ?o ?g. }

• W3176202430 endingPage "4784" @default.
• W3176202430 startingPage "4780" @default.
• W3176202430 abstract "Abstract Despite outstanding accomplishments in catalyst discovery, finding new, more efficient, environmentally neutral, and noble metal-free catalysts remains challenging and unsolved. Recently, complex solid solutions consisting of at least five different elements and often named as high-entropy alloys have emerged as a new class of electrocatalysts for a variety of reactions. The multicomponent combinations of elements facilitate tuning of active sites and catalytic properties. Predicting optimal catalyst composition remains difficult, making testing of a very high number of them indispensable. We present the high-throughput screening of the electrochemical activity of thin film material libraries prepared by combinatorial co-sputtering of metals which are commonly used in catalysis (Pd, Cu, Ni) combined with metals which are not commonly used in catalysis (Ti, Hf, Zr). Introducing unusual elements in the search space allows discovery of catalytic activity for hitherto unknown compositions. Material libraries with very similar composition spreads can show different activities vs. composition trends for different reactions. In order to address the inherent challenge of the huge combinatorial material space and the inability to predict active electrocatalyst compositions, we developed a high-throughput process based on co-sputtered material libraries, and performed high-throughput characterization using energy dispersive X-ray spectroscopy (EDS), scanning transmission electron microscopy (SEM), X-ray diffraction (XRD) and conductivity measurements followed by electrochemical screening by means of a scanning droplet cell. The results show surprising material compositions with increased activity for the oxygen reduction reaction and the hydrogen evolution reaction. Such data are important input data for future data-driven materials prediction." @default.
• W3176202430 created "2021-07-05" @default.
• W3176202430 creator A5023656866 @default.
• W3176202430 creator A5035321019 @default.
• W3176202430 creator A5048192399 @default.
• W3176202430 creator A5063123925 @default.
• W3176202430 creator A5067459856 @default.
• W3176202430 creator A5088354669 @default.
• W3176202430 date "2021-07-01" @default.
• W3176202430 modified "2023-10-14" @default.
• W3176202430 title "Searching novel complex solid solution electrocatalysts in unconventional element combinations" @default.
• W3176202430 cites W1965783559 @default.
• W3176202430 cites W1968985108 @default.
• W3176202430 cites W2007007768 @default.
• W3176202430 cites W2012283609 @default.
• W3176202430 cites W2023361558 @default.
• W3176202430 cites W2060742044 @default.
• W3176202430 cites W2201563651 @default.
• W3176202430 cites W2344967718 @default.
• W3176202430 cites W2618707089 @default.
• W3176202430 cites W2795185600 @default.
• W3176202430 cites W2806677418 @default.
• W3176202430 cites W2883326306 @default.
• W3176202430 cites W2896511002 @default.
• W3176202430 cites W2909236073 @default.
• W3176202430 cites W2914573344 @default.
• W3176202430 cites W2939390891 @default.
• W3176202430 cites W2945552497 @default.
• W3176202430 cites W2951644190 @default.
• W3176202430 cites W2960059926 @default.
• W3176202430 cites W2972052805 @default.
• W3176202430 cites W2980165457 @default.
• W3176202430 cites W2996421114 @default.
• W3176202430 cites W2999482379 @default.
• W3176202430 cites W3020204536 @default.
• W3176202430 cites W3048912808 @default.
• W3176202430 cites W3113875876 @default.
• W3176202430 doi "https://doi.org/10.1007/s12274-021-3637-z" @default.
• W3176202430 hasPublicationYear "2021" @default.
• W3176202430 type Work @default.
• W3176202430 sameAs 3176202430 @default.
• W3176202430 citedByCount "11" @default.
• W3176202430 countsByYear W31762024302022 @default.
• W3176202430 countsByYear W31762024302023 @default.
• W3176202430 crossrefType "journal-article" @default.
• W3176202430 hasAuthorship W3176202430A5023656866 @default.
• W3176202430 hasAuthorship W3176202430A5035321019 @default.
• W3176202430 hasAuthorship W3176202430A5048192399 @default.
• W3176202430 hasAuthorship W3176202430A5063123925 @default.
• W3176202430 hasAuthorship W3176202430A5067459856 @default.
• W3176202430 hasAuthorship W3176202430A5088354669 @default.
• W3176202430 hasBestOaLocation W31762024301 @default.
• W3176202430 hasConcept C127413603 @default.
• W3176202430 hasConcept C146088050 @default.
• W3176202430 hasConcept C147789679 @default.
• W3176202430 hasConcept C161790260 @default.
• W3176202430 hasConcept C171250308 @default.
• W3176202430 hasConcept C17525397 @default.
• W3176202430 hasConcept C178790620 @default.
• W3176202430 hasConcept C185592680 @default.
• W3176202430 hasConcept C192562407 @default.
• W3176202430 hasConcept C193016168 @default.
• W3176202430 hasConcept C2775871042 @default.
• W3176202430 hasConcept C2780841128 @default.
• W3176202430 hasConcept C33989665 @default.
• W3176202430 hasConcept C42360764 @default.
• W3176202430 hasConcept C52859227 @default.
• W3176202430 hasConceptScore W3176202430C127413603 @default.
• W3176202430 hasConceptScore W3176202430C146088050 @default.
• W3176202430 hasConceptScore W3176202430C147789679 @default.
• W3176202430 hasConceptScore W3176202430C161790260 @default.
• W3176202430 hasConceptScore W3176202430C171250308 @default.
• W3176202430 hasConceptScore W3176202430C17525397 @default.
• W3176202430 hasConceptScore W3176202430C178790620 @default.
• W3176202430 hasConceptScore W3176202430C185592680 @default.
• W3176202430 hasConceptScore W3176202430C192562407 @default.
• W3176202430 hasConceptScore W3176202430C193016168 @default.
• W3176202430 hasConceptScore W3176202430C2775871042 @default.
• W3176202430 hasConceptScore W3176202430C2780841128 @default.
• W3176202430 hasConceptScore W3176202430C33989665 @default.
• W3176202430 hasConceptScore W3176202430C42360764 @default.
• W3176202430 hasConceptScore W3176202430C52859227 @default.
• W3176202430 hasIssue "6" @default.
• W3176202430 hasLocation W31762024301 @default.
• W3176202430 hasLocation W31762024302 @default.
• W3176202430 hasLocation W31762024303 @default.
• W3176202430 hasLocation W31762024304 @default.
• W3176202430 hasOpenAccess W3176202430 @default.
• W3176202430 hasPrimaryLocation W31762024301 @default.
• W3176202430 hasRelatedWork W2010872403 @default.
• W3176202430 hasRelatedWork W2131631219 @default.
• W3176202430 hasRelatedWork W2182465065 @default.
• W3176202430 hasRelatedWork W2375410627 @default.
• W3176202430 hasRelatedWork W2472735067 @default.
• W3176202430 hasRelatedWork W2538310798 @default.
• W3176202430 hasRelatedWork W2613970801 @default.
• W3176202430 hasRelatedWork W2895938959 @default.
• W3176202430 hasRelatedWork W3054872367 @default.

• next