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- W3176335034 endingPage "150445" @default.
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- W3176335034 abstract "The low-concentration HCHO removal at room temperature is still a challenge in the indoor air purifying. Manganese dioxide catalyst (MnO2-M) derived from metal-organic frameworks (MOF) was synthesized via facile in-situ redox reaction. The obtained MnO2-M catalyst displayed superior activity and stability for low-concentration HCHO removal, reaching ~95% for 1.0 mg/m3 of HCHO under dynamic test mode and degrading 93.1% for 1.0 mg/m3 HCHO in 3 h under static test mode at room temperature. Moreover, the enhanced activity of MnO2-M could be attributed to the abundant chemisorbed oxygen species, numerous Mn-vacancies and proper pore size distribution. More crucially, the chemisorbed oxygen species on the MnO2-M could be rapidly activated by the transferable electrons and vacancies, thus significantly promoting the formation of reactive oxygen species and HCHO decomposition. The present work provides a new strategy to develop efficient catalyst for indoor air purification." @default.
- W3176335034 created "2021-07-05" @default.
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- W3176335034 date "2021-11-01" @default.
- W3176335034 modified "2023-10-13" @default.
- W3176335034 title "Metal organic frameworks derived manganese dioxide catalyst with abundant chemisorbed oxygen and defects for the efficient removal of gaseous formaldehyde at room temperature" @default.
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- W3176335034 doi "https://doi.org/10.1016/j.apsusc.2021.150445" @default.
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