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• W3176834597 endingPage "31050" @default.
• W3176834597 startingPage "31038" @default.
• W3176834597 abstract "The current work presents a facile and green synthesis of carbon quantum dots (C-dots), which could serve as initiators for polymerization. Herein, C-dots have been synthesized from an easily available green herb, dill leaves, by a single-step hydrothermal method. These C-dots were efficiently utilized as initiators for the photopolymerization of the polymer poly(norepinephrine) (PNE) for the first time. The photopolymerization is discussed by a factorial design, and the optimized synthesis conditions were evaluated by a third-order regression model of three reaction parameters: monomer concentration, C-dots concentration, and UV exposure time. The sign convention of the factorial design mode indicated that monomer concentration and time of exposure are the most important factors for polymerization. The photopolymerized poly(norepinephrine) was extensively studied using Fourier transform infrared (FTIR) analysis, X-ray photoelectron spectroscopy (XPS), mass spectra, scanning electron microscopy (SEM), atomic force microscopy (AFM), contact angle measurement, and thermogravimetric analysis (TGA). UV-assisted deposition of PNE on six different types of substrates was performed, and their water contact angle and surface morphology were studied to evaluate the coating. This UV-triggered polymerization technique was further applied to fabricate sandwich-like composite catalyst MXene/poly(norepinephrine)/copper nanoparticles. This catalyst displayed good performance in the reduction of 4-NP (4-nitrophenol) at ambient temperature, and the first-order rate constant of the catalysis was 9.39 × 10–3 s–1. The reusability of the catalyst was evaluated in terms of the conversion factor. After 10 catalytic cycles, the conversion to catalyze 4-NP was still greater than 91%. The catalytic performance was also evaluated in the continuous flow condition through a membrane, fabricated from a cellulose filter paper coated with MXene/poly(norepinephrine)/copper nanoparticles. This composite catalyst not only offers a practical mode for the catalytic reaction of MXene-based materials but also lays down the foundation for the development of new catalysts." @default.
• W3176834597 created "2021-07-05" @default.
• W3176834597 creator A5031590812 @default.
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• W3176834597 date "2021-06-25" @default.
• W3176834597 modified "2023-10-18" @default.
• W3176834597 title "Carbon-Dots-Initiated Photopolymerization: An <i>In Situ</i> Synthetic Approach for MXene/Poly(norepinephrine)/Copper Hybrid and its Application for Mitigating Water Pollution" @default.
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• W3176834597 doi "https://doi.org/10.1021/acsami.1c08111" @default.
• W3176834597 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34167297" @default.
• W3176834597 hasPublicationYear "2021" @default.
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