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- W3176840619 abstract "Here, we have demonstrated X-ray absorption spectroscopy, synchrotron X-ray diffraction, and Raman scattering studies on Cr-doped PrFeO3 ceramics and have proposed a possible correlation between the Goldschmidt structural tolerance factor, structural bandwidth, and eg electron bandwidth. It has been observed that these parameters scale in a similar fashion with Cr content, which infers the governance of these parameters by a common factor. Soft XAS experiments performed at Fe L-edge and O K-edge suggest the enhancement in overlapping between Fe 3d–O 2p orbitals, which results in an increase in the values of the eg electron bandwidth. Furthermore, with the help of strong experimental and theoretical evidence on the same samples, a mechanism in terms of orbital-facilitated charge transfer from Cr3+–O2––Fe3+ has been proposed. The importance of this mechanism lies in the fact that the Raman mode generated around 660 cm–1 may provide qualitative information about Δ, which is completely a new approach toward the information related to Δ. Thus, with the help of different experimental techniques, a correlation between the Goldschmidt structural tolerance factor, structural bandwidth, and eg electron bandwidth has been established." @default.
- W3176840619 created "2021-07-05" @default.
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- W3176840619 date "2021-06-17" @default.
- W3176840619 modified "2023-09-24" @default.
- W3176840619 title "Investigations on the Electronic Structure of the Strongly Correlated Electron System Cr-Doped PrFeO<sub>3</sub>" @default.
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- W3176840619 doi "https://doi.org/10.1021/acs.jpcc.1c02719" @default.
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