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- W3178203277 abstract "Developing highly active and durable electrocatalysts, consisting of earth-abundant elements, for oxygen evolution reaction (OER) is pivotal for large-scale water splitting for hydrogen production. Herein, we report that the commercially available FeNiCo alloy can be converted to a highly active electrocatalyst for OER by galvanostatic anodizing in a fluoride-containing ethylene glycol electrolyte. Anodizing of the alloy develops a porous film consisting of the (FeNiCo)F2 phase, which is readily converted to a highly active porous oxyhydroxide during anodic polarization in a KOH electrolyte. The anodized alloy exhibits high activity and high durability for OER with an overpotential as low as 0.26 V at a current density of 10 mA cm–2. The present study demonstrates that a simple and cost-effective anodizing process can be used to form a highly active OER electrode from a low-cost, practical, iron-based alloy. In addition, we found that fluorides containing Fe, Ni, and Co are excellent precursors for the formation of oxyhydroxides exhibiting high OER activity and durability." @default.
- W3178203277 created "2021-07-19" @default.
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- W3178203277 date "2021-07-07" @default.
- W3178203277 modified "2023-09-30" @default.
- W3178203277 title "Highly Active and Durable FeNiCo Oxyhydroxide Oxygen Evolution Reaction Electrocatalysts Derived from Fluoride Precursors" @default.
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- W3178203277 doi "https://doi.org/10.1021/acssuschemeng.1c03116" @default.
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