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- W3178758384 abstract "Ammonia (NH3) is one of the most important building blocks of the chemical industry and a promising sustainable energy carrier. Conventional production of NH3 via the Haber-Bosch process requires high temperature and high pressure, which is energy demanding and suffers safety issues. Photocatalytic nitrogen reduction reaction (NRR) is a green and sustainable route for NH3 production, and has been expected to be an alternative for NH3 production under mild conditions. However, solar-driven N2 activated has appeared as the bottleneck for photocatalytic NRR. In this work, we propose that single Ru atom supported by BeO monolayer is a promising photocatalytic single atom catalyst (SAC) for efficient N2 activation with visible illumination. The high efficiency originates from the enhanced absorption in the visible range, as well as the back-donation mechanism when N2 were adsorbed on the SAC. Our results show that N2 can be efficiently activated by the Ru/BeO SAC and be reduced to NH3 with extremely low limiting potential of −0.41 V. The NRR process also exhibits dominate selectivity respect to hydrogen evolution." @default.
- W3178758384 created "2021-07-19" @default.
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- W3178758384 date "2022-01-01" @default.
- W3178758384 modified "2023-10-10" @default.
- W3178758384 title "Highly efficient photocatalytic reduction of nitrogen into ammonia by single Ru atom catalyst supported by BeO monolayer" @default.
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- W3178758384 doi "https://doi.org/10.1016/j.cclet.2021.06.077" @default.
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