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• W3179196012 abstract "Two major subclasses of mononuclear non-heme ferrous enzymes use two electron-donating organic cofactors (α-ketoglutarate or pterin) to activate O2 to form FeIV═O intermediates that further react with their substrates through hydrogen atom abstraction or electrophilic aromatic substitution. New spectroscopic methodologies have been developed, enabling the study of the active sites in these enzymes and their oxygen intermediates. Coupled to electronic structure calculations, the results of these spectroscopies provide fundamental insight into mechanism. This Perspective summarizes the results of these studies in elucidating the mechanism of dioxygen activation to form the FeIV═O intermediate and the geometric and electronic structure of this intermediate that enables its high reactivity and selectivity in product formation." @default.
• W3179196012 created "2021-07-19" @default.
• W3179196012 creator A5024342453 @default.
• W3179196012 creator A5050139165 @default.
• W3179196012 creator A5071348965 @default.
• W3179196012 date "2021-07-16" @default.
• W3179196012 modified "2023-10-17" @default.
• W3179196012 title "Mechanisms of O₂ Activation by Mononuclear Non-Heme Iron Enzymes" @default.
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• W3179196012 doi "https://doi.org/10.1021/acs.biochem.1c00370" @default.
• W3179196012 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34266238" @default.
• W3179196012 hasPublicationYear "2021" @default.
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