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• W3179990144 abstract "• A novel synthetic route from BiOI to Bi 4 O 5 Br x I 2-x was designed. • The multiple coordinated strategy provided a good reference for the adjusting IEF of BiOX. • The confinement of positive and negative alternating atomic layers could provide some insights. • The possible morphology transformation and carbon-doped transfer were proposed. • A parallel attack mechanism of O 2 − and h + was proposed. Bi 4 O 5 Br x I 2-x C y solid solutions with simultaneous bismuth-enriched and low temperature homogeneous C doping were obtained by the phase crystal reforming of BiOI with solvothermal alkali assisted molten salt method. The internal electric field between alternating atomic layers was significantly enhanced due to the synergism of formation of solid solutions, enrichment Bi and homogeneous C doping. Driven by the strong internal electric field, the photogenerated electrons and holes of Bi 2.8 C 1.2 O 5 Br 0.5 I 1.5 were confined to the [Bi 2.8 C 1.2 O 5 ] 2+ layer and the double [Br 0.5 I 1.5 ] − layer, respectively, then effective separation of charge carriers was achieved. The removal rates over Bi 2.8 C 1.2 O 5 Br 0.5 I 1.5 of phenol, 4-chlorophenol, resorcinol and hydroquinone were 100 % in 1 h under visible light irradiation, which followed the parallel attack mechanism of O 2- and h + . This study provided a reference for the multiple coordinated regulation of internal electric field by formation of solid solutions, enrichment Bi and homogeneous doping." @default.
• W3179990144 created "2021-07-19" @default.
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• W3179990144 date "2021-12-01" @default.
• W3179990144 modified "2023-10-14" @default.
• W3179990144 title "Accurate guided alternating atomic layer enhance internal electric field to steering photogenerated charge separation for enhance photocatalytic activity" @default.
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• W3179990144 doi "https://doi.org/10.1016/j.apcatb.2021.120536" @default.
• W3179990144 hasPublicationYear "2021" @default.
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