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- W3182037618 abstract "Abstract An oxidative NHC‐catalyzed kinetic resolution (KR) of racemic mixtures is presented. The developed reaction furnishes tricyclic dihydropyranones with three contiguous stereocenters in excellent dia‐ and enantioselectivity, with good‐to‐moderate yields. Mechanistic studies indicate that the rate‐determining step of the reaction is the formation of the Breslow intermediate, while the selectivity determining step occurs later in the mechanism. The presented methodology enables rapid synthesis of complex structures in a single step." @default.
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- W3182037618 date "2021-07-06" @default.
- W3182037618 modified "2023-10-17" @default.
- W3182037618 title "Asymmetric Synthesis of Dihydropyranones with Three Contiguous Stereocenters by an NHC‐Catalyzed Kinetic Resolution" @default.
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- W3182037618 doi "https://doi.org/10.1002/ejoc.202100491" @default.
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