Matches in SemOpenAlex for { <https://semopenalex.org/work/W3182069823> ?p ?o ?g. }
- W3182069823 endingPage "12064" @default.
- W3182069823 startingPage "12056" @default.
- W3182069823 abstract "Aluminum fluoride (AlF3)-modified HZSM-5 obtained by simple mechanical mixing and calcination was used to enhance the conversion of the lignite pyrolysis volatiles to light aromatics. The results revealed that the appropriate amount of AlF3 modification can simultaneously dealuminize and aluminize to enhance the catalytic performance, in which dealumination considerably enlarged the pores while realumination generated more midstrength acid sites to compensate for the loss of acid sites caused by dealumination. HZ-2 (HZSM-5 mixed with 2 wt % AlF3) obtained the maximum light aromatics yield of 31.0 mg/g as a result of its abundant mesopores and suitable midstrength acid sites, especially the yield of benzene increased by 6.3 mg/g in comparison with that of the original HZSM-5. However, mixing with only a small amount of AlF3 generated the most serious carbon depositions because of the acidity enhancement by the critical role of alumination. Moreover, excessive AlF3 etched more framework Al that dramatically reduced the midstrength acid sites, inhibiting the formation of light aromatics, although the enlargement of pore size facilitated mass transfer. This one-step modification combining the expansion of the pore size and the optimization of acid sites provides a promising strategy for upgrading the lignite pyrolysis volatiles." @default.
- W3182069823 created "2021-07-19" @default.
- W3182069823 creator A5004177750 @default.
- W3182069823 creator A5017502093 @default.
- W3182069823 creator A5044479512 @default.
- W3182069823 creator A5044555512 @default.
- W3182069823 creator A5053184345 @default.
- W3182069823 creator A5055779145 @default.
- W3182069823 creator A5057061842 @default.
- W3182069823 creator A5060607066 @default.
- W3182069823 creator A5081766754 @default.
- W3182069823 creator A5089192549 @default.
- W3182069823 date "2021-07-14" @default.
- W3182069823 modified "2023-09-26" @default.
- W3182069823 title "Catalytic Upgrading of Lignite Pyrolysis Volatiles over AlF<sub>3</sub>-Modified HZSM-5 to Light Aromatics: Synergistic Effects of One-Step Dealumination and Realumination" @default.
- W3182069823 cites W1575041646 @default.
- W3182069823 cites W1826655 @default.
- W3182069823 cites W1968852536 @default.
- W3182069823 cites W1970724077 @default.
- W3182069823 cites W1980704616 @default.
- W3182069823 cites W1984527766 @default.
- W3182069823 cites W1989599087 @default.
- W3182069823 cites W2005305006 @default.
- W3182069823 cites W2032621257 @default.
- W3182069823 cites W2032876097 @default.
- W3182069823 cites W2040450726 @default.
- W3182069823 cites W2042327736 @default.
- W3182069823 cites W2051687776 @default.
- W3182069823 cites W2081661880 @default.
- W3182069823 cites W2086021669 @default.
- W3182069823 cites W2123635631 @default.
- W3182069823 cites W2177207920 @default.
- W3182069823 cites W2328934072 @default.
- W3182069823 cites W2342876394 @default.
- W3182069823 cites W2513553109 @default.
- W3182069823 cites W2554831430 @default.
- W3182069823 cites W2605677372 @default.
- W3182069823 cites W2707933576 @default.
- W3182069823 cites W2737735636 @default.
- W3182069823 cites W2748072851 @default.
- W3182069823 cites W2774744751 @default.
- W3182069823 cites W2784121221 @default.
- W3182069823 cites W2790691955 @default.
- W3182069823 cites W2796359415 @default.
- W3182069823 cites W2808675721 @default.
- W3182069823 cites W2884773989 @default.
- W3182069823 cites W2908985158 @default.
- W3182069823 cites W2914708340 @default.
- W3182069823 cites W2957552637 @default.
- W3182069823 cites W2975661039 @default.
- W3182069823 cites W2979524383 @default.
- W3182069823 cites W2986683731 @default.
- W3182069823 cites W2987786882 @default.
- W3182069823 cites W2993827226 @default.
- W3182069823 cites W3001880539 @default.
- W3182069823 cites W3003586592 @default.
- W3182069823 cites W3015895178 @default.
- W3182069823 cites W3033036347 @default.
- W3182069823 cites W3040066372 @default.
- W3182069823 cites W3088163569 @default.
- W3182069823 cites W3120322739 @default.
- W3182069823 cites W3135030180 @default.
- W3182069823 cites W771553119 @default.
- W3182069823 doi "https://doi.org/10.1021/acs.energyfuels.1c01633" @default.
- W3182069823 hasPublicationYear "2021" @default.
- W3182069823 type Work @default.
- W3182069823 sameAs 3182069823 @default.
- W3182069823 citedByCount "6" @default.
- W3182069823 countsByYear W31820698232022 @default.
- W3182069823 countsByYear W31820698232023 @default.
- W3182069823 crossrefType "journal-article" @default.
- W3182069823 hasAuthorship W3182069823A5004177750 @default.
- W3182069823 hasAuthorship W3182069823A5017502093 @default.
- W3182069823 hasAuthorship W3182069823A5044479512 @default.
- W3182069823 hasAuthorship W3182069823A5044555512 @default.
- W3182069823 hasAuthorship W3182069823A5053184345 @default.
- W3182069823 hasAuthorship W3182069823A5055779145 @default.
- W3182069823 hasAuthorship W3182069823A5057061842 @default.
- W3182069823 hasAuthorship W3182069823A5060607066 @default.
- W3182069823 hasAuthorship W3182069823A5081766754 @default.
- W3182069823 hasAuthorship W3182069823A5089192549 @default.
- W3182069823 hasConcept C104779481 @default.
- W3182069823 hasConcept C121332964 @default.
- W3182069823 hasConcept C127413603 @default.
- W3182069823 hasConcept C134121241 @default.
- W3182069823 hasConcept C138777275 @default.
- W3182069823 hasConcept C140205800 @default.
- W3182069823 hasConcept C159985019 @default.
- W3182069823 hasConcept C161790260 @default.
- W3182069823 hasConcept C178790620 @default.
- W3182069823 hasConcept C179104552 @default.
- W3182069823 hasConcept C185592680 @default.
- W3182069823 hasConcept C192562407 @default.
- W3182069823 hasConcept C2777691172 @default.
- W3182069823 hasConcept C2778077586 @default.
- W3182069823 hasConcept C2781047139 @default.
- W3182069823 hasConcept C36759035 @default.
- W3182069823 hasConcept C42360764 @default.