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- W3182282169 abstract "A facile strategy is applied to construct Fe supported ZSM-5 (Fe/HZ5-HTS) via hydrothermal post-treatment and applied to ethane non-oxidative dehydrogenation. Compared with Fe/HZ5-IWI prepared by incipient wetness impregnation, Fe/HZ5-HTS exhibits superior catalytic activity and long catalyst stability with 6000 minutes time-on-stream. An obvious volcanic curve is observed between the ethylene generation rate and Fe content, and 1.0Fe/HZ5-HTS exhibits the highest ethylene generation rate with 0.166 mmol C2H4 s−1 gFe−1 over different Fe loading, which is twice as much as that of 1.0Fe/HZ5-IWI. According to various characterizations, isolated Fe3+ species and carburized Fe species are active sites, and the better catalytic performance over 1.0Fe/HZ5-HTS is ascribed to more disperse Fe species and exposing more Fe species in the surface. Besides, the lower ethylene desorption temperature and higher ethane desorption temperature over Fe/HZ5-HTS could suppress the overreaction of the ethylene to generate coke and increase ethane residence reaction time, resulting in less coke deposition and facilitating the catalytic performance." @default.
- W3182282169 created "2021-07-19" @default.
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- W3182282169 date "2021-07-28" @default.
- W3182282169 modified "2023-10-18" @default.
- W3182282169 title "Enhanced Catalytic Performance of Fe‐containing HZSM‐5 for Ethane Non‐Oxidative Dehydrogenation via Hydrothermal Post‐Treatment" @default.
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- W3182282169 doi "https://doi.org/10.1002/cctc.202100752" @default.
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