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• W3183772201 abstract "Solid amine adsorbents cannot typically maintain desirable CO2 capture capacity while having ultralow regeneration temperatures. To address this issue, a novel thermoresponsive nanofiber-based solid amine adsorbent (TRCNF/PEIA) with high amino density and high content of thermoresponsive intelligent groups was designed and prepared using epichlorohydrin to rapidly cross-link polyethyleneimine (PEI) and a thermoresponsive cellulose nanofiber (TRCNF). The latter was obtained by grafting N-isopropylacrylamide (NIPAm) on the cellulose nanofiber (CNF) through Ce (IV)-initiated free radical polymerization. The as-prepared TRCNF/PEIA simultaneously showed high capture capacity (6.74 mmol/g) with water at 25 °C and a low regeneration temperature (60 °C). A comparison of the adsorption–desorption properties of TRCNF/PEIA with those of the PEIA, which was prepared using a procedure similar to that of TRCNF/PEIA but without TRCNF, showed that the thermoresponsive property of PNIPAm and the synergy of the hydroxyl groups of TRCNF/PEIA could facilitate CO2 complete desorption from the adsorbent at 60 °C, which was the lowest regeneration temperature to maintain the high adsorption capacity (≥6 mmol/g) of the adsorbents, based on the literature reports." @default.
• W3183772201 created "2021-08-02" @default.
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• W3183772201 date "2021-07-20" @default.
• W3183772201 modified "2023-10-16" @default.
• W3183772201 title "Design of an Intelligent Nanofiber-Based Solid Amine Adsorbent with High CO₂ Capture Capacity and an Ultralow Regeneration Temperature" @default.
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• W3183772201 doi "https://doi.org/10.1021/acssuschemeng.1c02387" @default.
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