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• W3184569862 abstract "The formation of polymer-patch nanoparticles (PNPs) involves a condensation process of grafted chains on a nanoparticle (NP) surface, which is conventionally achieved via a fine-tuning of the solvent quality. However, such a critical solvent condition differs dramatically between polymers, and the formation mechanism of different patchy structures remains under debate. In this study, we demonstrate by a combined simulation and experimental study that such a surface-patterning process can be easily achieved via a simple solvent evaporation process, which creates a natural nonsolvent condition and is, in principle, adaptable for all polymers. More importantly, we find that patchy structures are controlled by a delicate balance between enthalpic interaction and the entropy penalty of grafted chains. A small variation of cohesive energy density can lead to a dramatic change in patch structure. This work offers a robust yet easy approach for the fabrication of PNPs and provides new insights into polymer segregation on spherical surfaces." @default.
• W3184569862 created "2021-08-02" @default.
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• W3184569862 date "2021-07-22" @default.
• W3184569862 modified "2023-10-14" @default.
• W3184569862 title "Solvent-Evaporation Induced and Mechanistic Entropy-Enthalpy-Balance Controlled Polymer Patch Formation on Nanoparticle Surfaces" @default.
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• W3184569862 doi "https://doi.org/10.1021/acs.jpclett.1c01979" @default.
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• W3184569862 hasPublicationYear "2021" @default.
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