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• W3185417044 endingPage "161203" @default.
• W3185417044 startingPage "161203" @default.
• W3185417044 abstract "• The layered MOF-71 is used as precursor to synthesis Co-CoP/C material. • The Co-CoP/C@S electrode presents excellent electrochemical performance. • Exploring the catalytic effect of CoP on lithium polysulfides. The commercialization of lithium-sulfur (Li-S) batteries is severely plagued by the shuttle effect and sluggish kinetic conversion of polysulfides. Herein, the layered cobalt phosphide CoP/C nanoparticle derived from MOF-71 by two-step heat treatment was synthesized to act as sulfur host in Li-S batteries. The physical characterization results indicate that Co-CoP/C has a specific surface area of 113 m 2 g −1 , with more micropores and mesopores, which is beneficial to the transmission of ions and electrons. MOF-derived polar metal phosphide Co-CoP/C has shown layered porous structure, which can provide more the active site to adsorb more polysulfides, furthermore, the cobalt phosphide can promote catalytic conversion of polysulfides. Thus the lithium-sulfur battery assembled with Co-CoP/C@S as the positive electrode showed excellent electrochemical performance: tested at a rate of 0.2 C, the initial discharge specific capacity of the battery reached 1441.9 mAh g −1 . Additionally, the long-cycle stability performance test was performed at a rate of 0.5 C, and the battery still maintained a reversible specific capacity above 600 mAh g −1 after 300 cycles of charge and discharge." @default.
• W3185417044 created "2021-08-02" @default.
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• W3185417044 date "2021-12-01" @default.
• W3185417044 modified "2023-10-01" @default.
• W3185417044 title "MOF-71 derived layered Co-CoP/C for advanced Li-S batteries" @default.
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• W3185417044 doi "https://doi.org/10.1016/j.jallcom.2021.161203" @default.
• W3185417044 hasPublicationYear "2021" @default.
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