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• W3185443695 startingPage "11325" @default.
• W3185443695 abstract "Photoinduced in situ oxidation of half-sandwich metal complexes to high-valent cationic metal complexes has been used to accelerate catalytic reactions. Here, we report the unprecedented photoinduced in situ reduction of half-sandwich metal [Rh(III)] complexes to low-valent anionic metal [Rh(II)] ate complexes, which facilitate ligand exchange with electron-deficient elements (diboron). This strategy was realized by using a functionalized cyclopentadienyl (CpA3) Rh(III) catalyst we developed, which enabled the basic group-directed room temperature ortho-C-H borylation of arenes." @default.
• W3185443695 created "2021-08-02" @default.
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• W3185443695 date "2021-07-20" @default.
• W3185443695 modified "2023-10-14" @default.
• W3185443695 title "Photo-Induced <i>ortho</i>-C–H Borylation of Arenes through In Situ Generation of Rhodium(II) Ate Complexes" @default.
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• W3185443695 doi "https://doi.org/10.1021/jacs.1c05859" @default.
• W3185443695 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34283597" @default.
• W3185443695 hasPublicationYear "2021" @default.
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