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• W3186293625 abstract "Abstract Nickel aluminum layered double hydroxide (NiAl LDH) with nitrate in its interlayer is investigated as a negative electrode material for lithium-ion batteries (LIBs). The effect of the potential range (i.e., 0.01–3.0 V and 0.4–3.0 V vs. Li + /Li) and of the binder on the performance of the material is investigated in 1 M LiPF 6 in EC/DMC vs. Li. The NiAl LDH electrode based on sodium alginate (SA) binder shows a high initial discharge specific capacity of 2586 mAh g −1 at 0.05 A g −1 and good stability in the potential range of 0.01–3.0 V vs. Li + /Li, which is better than what obtained with a polyvinylidene difluoride (PVDF)-based electrode. The NiAl LDH electrode with SA binder shows, after 400 cycles at 0.5 A g −1 , a cycling retention of 42.2% with a capacity of 697 mAh g −1 and at a high current density of 1.0 A g −1 shows a retention of 27.6% with a capacity of 388 mAh g −1 over 1400 cycles. In the same conditions, the PVDF-based electrode retains only 15.6% with a capacity of 182 mAh g −1 and 8.5% with a capacity of 121 mAh g −1 , respectively. Ex situ X-ray photoelectron spectroscopy (XPS) and ex situ X-ray absorption spectroscopy (XAS) reveal a conversion reaction mechanism during Li + insertion into the NiAl LDH material. X-ray diffraction (XRD) and XPS have been combined with the electrochemical study to understand the effect of different cutoff potentials on the Li-ion storage mechanism. Graphical abstract The as-prepared NiAl-NO 3 − -LDH with the rhombohedral R-3 m space group is investigated as a negative electrode material for lithium-ion batteries (LIBs). The effect of the potential range (i.e., 0.01–3.0 V and 0.4–3.0 V vs. Li + /Li) and of the binder on the material’s performance is investigated in 1 M LiPF 6 in EC/DMC vs. Li. Ex situ X-ray photoelectron spectroscopy (XPS) and ex situ X-ray absorption spectroscopy (XAS) reveal a conversion reaction mechanism during Li + insertion into the NiAl LDH material. X-ray diffraction (XRD) and XPS have been combined with the electrochemical study to understand the effect of different cutoff potentials on the Li-ion storage mechanism. This work highlights the possibility of the direct application of NiAl LDH materials as negative electrodes for LIBs." @default.
• W3186293625 created "2021-08-02" @default.
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• W3186293625 date "2021-07-21" @default.
• W3186293625 modified "2023-10-12" @default.
• W3186293625 title "Electrochemical study on nickel aluminum layered double hydroxides as high-performance electrode material for lithium-ion batteries based on sodium alginate binder" @default.
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• W3186293625 doi "https://doi.org/10.1007/s10008-021-05011-y" @default.
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