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• W3186331331 endingPage "7356" @default.
• W3186331331 startingPage "7350" @default.
• W3186331331 abstract "The high cost of noble metal catalysts has been a major factor limiting their industrial applications. It is thus of strong interest to develop catalysts with minimum metal loading. Here, we designed and prepared a single-atom ruthenium catalyst through a cascade anchoring strategy to maximize the efficiency of Ru atoms for acetylene hydrochlorination. The single-atom catalyst supported on commercial activated carbon (AC) exhibits excellent catalytic activity with acetylene conversion of 95.4% at an acetylene gas hourly space velocity (GHSV) of 720 h–1 and almost no deactivation during a 600 h catalyst lifetime test. In conjunction with a series of experimental characterizations of the catalyst, including aberration-corrected scanning transmission electron microscopy (Ac-STEM), X-ray photoelectron spectroscopy (XPS), and extended X-ray absorption fine spectroscopy (EXAFS), density functional theory (DFT) study shows that RuN4 sites are likely responsible for acetylene hydrochlorination catalytic activity. This work provides a strategy to design efficient single-atom catalysts for acetylene hydrochlorination and helps us to gain deeper understanding of single-atom catalytic mechanisms." @default.
• W3186331331 created "2021-08-02" @default.
• W3186331331 creator A5025867944 @default.
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• W3186331331 date "2021-07-29" @default.
• W3186331331 modified "2023-10-16" @default.
• W3186331331 title "Single-Atom Ruthenium Catalytic Sites for Acetylene Hydrochlorination" @default.
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• W3186331331 doi "https://doi.org/10.1021/acs.jpclett.1c01779" @default.
• W3186331331 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34324364" @default.
• W3186331331 hasPublicationYear "2021" @default.
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